David Le Bolloc’h

Research Director CNRS

Interests

  • Charge Density Wave phases
  • Sliding Processes and Soliton Lattices
  • Coherent X-ray diffraction
  • Free Electron Laser
  • Pinning and Deformations

Education

  • PhD « Order-Disorder in Condensed Matter » (Laboratoire Léon Brillouin CEA/LEM ONERA)
  • Post doctoral position (Université de Houston UofH, Texas) /Oak Ridge /NSLS Brookhaven N.Y.
  • Post doctoral position (ESRF Grenoble France)
  • Research associate, Laboratoire de Physique des Solides (LPS), université Paris-Saclay
  • Habilitation to supervise research (HDR), Université Paris-Saclay

Electronic crystals and coherence

Transport of charges through CDW shear

Electronic transport in CDW materials has been observed through the behavior of the underlying atomic lattice using an intense X-ray beam generated by a Free Electron Laser (XFEL). In charge density wave systems, the electrons and the atomic lattice exhibit a wave-like behavior, the two modulations being inseparable. This phase of matter is very sensitive to various external excitations, such as changes in temperature, an ultrashort laser pulse or even weak currents. In the latter case, when a direct current above a critical threshold is applied to the sample, an additional current appears in the crystal. It is naturally pulsed and is directly linked to the behavior of the CDW. This effect is explained by a CDW deformation under current, eventually breaking beyond a certain deformation limit and periodically releasing charged topological objects that travel over macroscopic distances. This phenomenon has been observed thanks to the coherent and extended X-ray beam generated from the LCLS XFEL source at Stanford. The CDW phase was deduced from the diffraction patterns by applying a genetic algorithm. The CDW exhibits astonishing spatial coherence despite its nanometer period. It continuously deforms from one edge of the crystal to the other, which is several tens of microns wide. Like a guitar string plucked at both ends that bends under the effect of a force, the wave bends under the effect of the current pinned by the two side surfaces of the crystal. This shearing effect increases as the current increases, then suddenly relaxes above the threshold current (see figure 1). The wave deforms in the transverse direction by shear but also in the longitudinal direction, like an accordion that contracts and expands (see figure 2). The two types of deformation, transverse and longitudinal, are closely coupled, with the relaxation of one above the threshold leading to the appearance of the other. In addition, the steps on the crystal surface also act as traps, preventing it from slipping (see the two arrows on Fig.1). This result illustrates the capabilities of the new XFEL sources which, combined with appropriate analysis methods, open up new perspectives for observing and understanding the behavior of electronic systems

The importance of shear on the collective charge transport in CDWs revealed by an XFEL source,

David Le Bolloc’h, Ewen Bellec, Darine Ghoneim, Antoine Gallo-Frantz https, Pawel Wzietek, Luc Ortega, Anders Madsen, Pierre Monceau, Mathieu Chollet, Isabel Gonzales-Vallejo, Vincent L. R. Jacques, and Aleksandr Sinchenko, Sci. Adv., 11, eadr6034 (2025)

Doi :10.1126/sciadv.adr6034

Archives ouvertes : hal-04864367v1

Highlight CNRS février 2025 : https://www.inp.cnrs.fr/fr/cnrsinfo/cisaillement-dune-onde-de-densite-de-charge-observe-par-une-source-xfel


Publication list on ResearchGate:

https://www.researchgate.net/profile/David-Le-Bolloch/research

Affichage des résultats 1 à 12 sur 43 au total
  • Article dans une revue

    David Le Bolloc’h, Ewen Bellec, Darine Ghoneim, Antoine Gallo-Frantz, Pawel Wzietek, et al.. The importance of shear on the collective charge transport in CDWs revealed by an XFEL source. Science Advances , 2025, 11, pp.eadr6034. ⟨10.1126/sciadv.adr6034⟩. ⟨hal-04864367⟩

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  • Article dans une revue

    Antoine Gallo--Frantz, V. Jacques, A. Sinchenko, D. Ghoneim, L. Ortega, et al.. Charge density waves tuned by biaxial tensile stress. Nature Communications, 2024, 15 (1), pp.3667. ⟨10.1038/s41467-024-47626-5⟩. ⟨hal-04569145v2⟩

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  • Pré-publication, Document de travail

    Ewen Bellec, Darine Ghoneim, Antoine Gallo, Vlr Jacques, Isabel Gonzalez-Vallejo, et al.. Charge Density Wave bending observed by Xfel source acting as a tunable electronic lens for hard x-rays. 2023. ⟨hal-04210398⟩

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  • Article dans une revue

    David Le Bolloc'h, Ewen Bellec, Natacha Kirova, Vincent L R Jacques. Tracking Defects of Electronic Crystals by Coherent X-ray Diffraction. Symmetry, 2023, 15 (7), pp.1449. ⟨10.3390/sym15071449⟩. ⟨hal-04251860⟩

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  • Article dans une revue

    Pierre Godard, Mariana Verezhak, Tarik Sadat, Florent Mignerot, Vincent Jacques, et al.. In situ compression of micropillars under coherent X-ray diffraction: a case study of experimental and data-analysis constraints. Journal of Applied Crystallography, 2023, 56 (2), pp.381-390. ⟨10.1107/S1600576723000493⟩. ⟨hal-04236916⟩

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  • Pré-publication, Document de travail

    David Le Bolloc’h, Ewen Bellec, Natacha Kirova, Vincent Jacques. Tracking defects of Electronic Crystals by Coherent X-ray Diffraction. 2023. ⟨hal-04050713⟩

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  • Article dans une revue

    Ewen Bellec, Vincent Jacques, Jonathan Caillaux, David Le Bolloc'H. The essential role of surface pinning in the dynamics of charge density waves submitted to external dc fields. The European Physical Journal B: Condensed Matter and Complex Systems, 2020, 93 (9), ⟨10.1140/epjb/e2020-10211-6⟩. ⟨hal-03088687⟩

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  • Article dans une revue

    E. Bellec, I. Gonzalez-Vallejo, V.L.R. Jacques, A. Sinchenko, A. Orlov, et al.. Evidence of charge density wave transverse pinning by x-ray microdiffraction. Physical Review B, 2020, 101 (12), pp.125122. ⟨10.1103/PhysRevB.101.125122⟩. ⟨hal-03085984⟩

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  • Article dans une revue

    Isabel González Vallejo, Geoffrey Gallé, Brice Arnaud, Shelley Scott, Max Lagally, et al.. Observation of large multiple scattering effects in ultrafast electron diffraction on monocrystalline silicon. Physical Review B, 2018, 97 (5), pp.54302. ⟨10.1103/PhysRevB.97.054302⟩. ⟨hal-03088683v2⟩

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  • Communication dans un congrès

    Min-I Lee, A N Barragán, M.N. Nair, V. Jacques, D. Le Bolloc'H, et al.. Experimental valence band dispersion of CH3NH3PbI3 hybrid organic-inorganic perovskite. 33rd European Conference On Surface Science (ECOSS 2017), Aug 2017, Szeged, Hungary. ⟨hal-01572155⟩

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  • Poster de conférence

    Min-I Lee, A Barragán, M.N. Nair, V. Jacques, D. Le Bolloc'H, et al.. k-resolved band structure of CH3NH3PbI3 hybrid organic-inorganic perovskite. 24ème Colloque Générale de la Société Française de Physique, Jul 2017, Orsay, France. . ⟨hal-01572183⟩

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  • Communication dans un congrès

    Min-I Lee, A. Barragan, M.N. Nair, Vincent Jacques, D. Le Bolloc'H, et al.. Effet de la transition de phase structurelle sur la structure de bande résolue en k de la pérovskite hybride organique-inorganique CH3NH3PbI3. Journée Surfaces et Interfaces, Jan 2017, Rennes, France. ⟨hal-01451013⟩

    Année de publication

    Disponible en libre accès

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